A photochromic main-chain liquid crystalline polymer and its photo-stimulated actuating properties

  • Myong Hoon Lee*
  • , Hyong J. Choi
  • , Kwang Un Jeong
  • , Liang Chy Chien
  • *Corresponding author for this work

Research output: Contribution to conferenceConference paperpeer-review

Abstract

To explore novel photoresponsive liquid crystalline polymer actuator, a new difunctional photosensitive nematic liquid crystalline monomer was synthesized synthesized in high yield (>60% overall), and polymerized via acyclic diene metathesis polymerization (ADMET) method. Nematic monomer, 4-butoxy-2'-(4-hex-5- enyloxy)-4'-(4-hex-5-enyloxybenzyloxy)-azobenzene, exhibited crystalline to nematic and nematic to isotropic transitions at 85.6 and 98.3°C, respectively. ADMET polymerization of the monomer using Grubbs catalyst (Gen II) was performed to obtain a high molecular weight polymer. Brown colored free-standing polymer film and fiber were prepared from casting chloroform solution or from drawing polymer melt, respectively. The polymer film showed nematic liquid crystalline property with photosensitive phase transition behavior as observed by polarized microscope and differential scanning calorimetry. The photomechanical deformation of the film and fiber induced by polarized UV irradiation was investigated.

Original languageEnglish
Title of host publicationEmerging Liquid Crystal Technologies III
DOIs
StatePublished - 2008
EventEmerging Liquid Crystal Technologies III - San Jose, CA, United States
Duration: 2008.01.202008.01.22

Publication series

NameProceedings of SPIE - The International Society for Optical Engineering
Volume6911
ISSN (Print)0277-786X

Conference

ConferenceEmerging Liquid Crystal Technologies III
Country/TerritoryUnited States
CitySan Jose, CA
Period08.01.2008.01.22

Keywords

  • LC polymer
  • Photo-actuator
  • Photochromic

Quacquarelli Symonds(QS) Subject Topics

  • Materials Science
  • Computer Science & Information Systems
  • Mathematics
  • Engineering - Electrical & Electronic
  • Engineering - Petroleum
  • Data Science
  • Physics & Astronomy

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