Development of pilot WGS/multi-layer membrane for CO 2 capture

See Hoon Lee; Jung Nam Kim; Won Hyun Eom; Shin Kun Ryi; Jong Soo Park; Il Hyun Baek

doi:10.1016/j.cej.2012.07.013

Development of pilot WGS/multi-layer membrane for CO ₂ capture

See Hoon Lee
, Jung Nam Kim
, Won Hyun Eom
, Shin Kun Ryi
, Jong Soo Park
, Il Hyun Baek^*

^*Corresponding author for this work

Major of Mineral Resources and Energy Engineering

Korea Institute of Energy Research

Research output: Contribution to journal › Journal article › peer-review

21 Scopus citations

Abstract

For pre-combustion CO ₂ capture processes, a 1Nm ³/h water gas shift (WGS)/multi-layer membrane system has been developed. Simulated syngas (H ₂: 25-35, CO: 60-65, CO ₂: 5-15 vol.%) was used in these experiments. The 1Nm ³/h WGS/multi-layer membrane system consisted of mass flow controllers, water gas shift reactors, gas/steam separators, five layer Pd-Cu membrane module, back pressure regulator, gas chromatograph (GC) analyzers and nondispersive infrared (ND-IR) gas analyzers. The operation conditions of WGS/multi-layer membrane system were 200-400°C, 10-20bar and steam/carbon ratios in WGS were between 2.0 and 5.0. In the experiments of WGS/multi-layer membrane system, the average gas concentration before membrane module was H ₂: 57-58, CO ₂: 42-43, CO: 0.2-0.3 vol.%. The CO ₂ concentration of retentate flow reached up to 80 vol.% and the H ₂ concentration of permeate flow was over 99 vol.%.

Original language	English
Pages (from-to)	521-525
Number of pages	5
Journal	Chemical Engineering Journal
Volume	207-208
DOIs	https://doi.org/10.1016/j.cej.2012.07.013
State	Published - 2012.10.1

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

SDG 13 Climate Action

Keywords

CO capture
Gasification
Membrane
Water gas shift (WGS)

Quacquarelli Symonds(QS) Subject Topics

Environmental Sciences
Engineering - Mechanical
Engineering - Petroleum
Engineering - Chemical
Chemistry

Access to Document

10.1016/j.cej.2012.07.013

Cite this

@article{1e2524d29a714ee3888c6ffe75c9f372,

title = "Development of pilot WGS/multi-layer membrane for CO 2 capture",

abstract = "For pre-combustion CO 2 capture processes, a 1Nm 3/h water gas shift (WGS)/multi-layer membrane system has been developed. Simulated syngas (H 2: 25-35, CO: 60-65, CO 2: 5-15 vol.\%) was used in these experiments. The 1Nm 3/h WGS/multi-layer membrane system consisted of mass flow controllers, water gas shift reactors, gas/steam separators, five layer Pd-Cu membrane module, back pressure regulator, gas chromatograph (GC) analyzers and nondispersive infrared (ND-IR) gas analyzers. The operation conditions of WGS/multi-layer membrane system were 200-400°C, 10-20bar and steam/carbon ratios in WGS were between 2.0 and 5.0. In the experiments of WGS/multi-layer membrane system, the average gas concentration before membrane module was H 2: 57-58, CO 2: 42-43, CO: 0.2-0.3 vol.\%. The CO 2 concentration of retentate flow reached up to 80 vol.\% and the H 2 concentration of permeate flow was over 99 vol.\%.",

keywords = "CO capture, Gasification, Membrane, Water gas shift (WGS)",

author = "Lee, \{See Hoon\} and Kim, \{Jung Nam\} and Eom, \{Won Hyun\} and Ryi, \{Shin Kun\} and Park, \{Jong Soo\} and Baek, \{Il Hyun\}",

year = "2012",

month = oct,

day = "1",

doi = "10.1016/j.cej.2012.07.013",

language = "English",

volume = "207-208",

pages = "521--525",

journal = "Chemical Engineering Journal",

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TY - JOUR

T1 - Development of pilot WGS/multi-layer membrane for CO 2 capture

AU - Lee, See Hoon

AU - Kim, Jung Nam

AU - Eom, Won Hyun

AU - Ryi, Shin Kun

AU - Park, Jong Soo

AU - Baek, Il Hyun

PY - 2012/10/1

Y1 - 2012/10/1

N2 - For pre-combustion CO 2 capture processes, a 1Nm 3/h water gas shift (WGS)/multi-layer membrane system has been developed. Simulated syngas (H 2: 25-35, CO: 60-65, CO 2: 5-15 vol.%) was used in these experiments. The 1Nm 3/h WGS/multi-layer membrane system consisted of mass flow controllers, water gas shift reactors, gas/steam separators, five layer Pd-Cu membrane module, back pressure regulator, gas chromatograph (GC) analyzers and nondispersive infrared (ND-IR) gas analyzers. The operation conditions of WGS/multi-layer membrane system were 200-400°C, 10-20bar and steam/carbon ratios in WGS were between 2.0 and 5.0. In the experiments of WGS/multi-layer membrane system, the average gas concentration before membrane module was H 2: 57-58, CO 2: 42-43, CO: 0.2-0.3 vol.%. The CO 2 concentration of retentate flow reached up to 80 vol.% and the H 2 concentration of permeate flow was over 99 vol.%.

AB - For pre-combustion CO 2 capture processes, a 1Nm 3/h water gas shift (WGS)/multi-layer membrane system has been developed. Simulated syngas (H 2: 25-35, CO: 60-65, CO 2: 5-15 vol.%) was used in these experiments. The 1Nm 3/h WGS/multi-layer membrane system consisted of mass flow controllers, water gas shift reactors, gas/steam separators, five layer Pd-Cu membrane module, back pressure regulator, gas chromatograph (GC) analyzers and nondispersive infrared (ND-IR) gas analyzers. The operation conditions of WGS/multi-layer membrane system were 200-400°C, 10-20bar and steam/carbon ratios in WGS were between 2.0 and 5.0. In the experiments of WGS/multi-layer membrane system, the average gas concentration before membrane module was H 2: 57-58, CO 2: 42-43, CO: 0.2-0.3 vol.%. The CO 2 concentration of retentate flow reached up to 80 vol.% and the H 2 concentration of permeate flow was over 99 vol.%.

KW - CO capture

KW - Gasification

KW - Membrane

KW - Water gas shift (WGS)

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U2 - 10.1016/j.cej.2012.07.013

DO - 10.1016/j.cej.2012.07.013

M3 - Journal article

AN - SCOPUS:84866869777

SN - 1385-8947

VL - 207-208

SP - 521

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JO - Chemical Engineering Journal

JF - Chemical Engineering Journal

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