Efficient Planar Perovskite Solar Cells Using Passivated Tin Oxide as an Electron Transport Layer

Yonghui Lee; Seunghwan Lee; Gabseok Seo; Sanghyun Paek; Kyung Taek Cho; Aron J. Huckaba; Marco Calizzi; Dong won Choi; Jin Seong Park; Dongwook Lee; Hyo Joong Lee; Abdullah M. Asiri; Mohammad Khaja Nazeeruddin

doi:10.1002/advs.201800130

Efficient Planar Perovskite Solar Cells Using Passivated Tin Oxide as an Electron Transport Layer

Yonghui Lee^*
, Seunghwan Lee
, Gabseok Seo
, Sanghyun Paek
, Kyung Taek Cho
, Aron J. Huckaba
, Marco Calizzi
, Dong won Choi
, Jin Seong Park
, Dongwook Lee
, Hyo Joong Lee
, Abdullah M. Asiri
, Mohammad Khaja Nazeeruddin

^*Corresponding author for this work

Department of Chemistry

Research output: Contribution to journal › Journal article › peer-review

151 Scopus citations

Abstract

Planar perovskite solar cells using low-temperature atomic layer deposition (ALD) of the SnO₂ electron transporting layer (ETL), with excellent electron extraction and hole-blocking ability, offer significant advantages compared with high-temperature deposition methods. The optical, chemical, and electrical properties of the ALD SnO₂ layer and its influence on the device performance are investigated. It is found that surface passivation of SnO₂ is essential to reduce charge recombination at the perovskite and ETL interface and show that the fabricated planar perovskite solar cells exhibit high reproducibility, stability, and power conversion efficiency of 20%.

Original language	English
Article number	1800130
Journal	Advanced Science
Volume	5
Issue number	6
DOIs	https://doi.org/10.1002/advs.201800130
State	Published - 2018.06

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

SDG 7 Affordable and Clean Energy

Keywords

atomic layer deposition
passivation
perovskites
planar perovskite solar cells
SnO electron transporting layers

Quacquarelli Symonds(QS) Subject Topics

Materials Science
Medicine
Engineering - Chemical
Physics & Astronomy
Biological Sciences

Access to Document

10.1002/advs.201800130

Cite this

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title = "Efficient Planar Perovskite Solar Cells Using Passivated Tin Oxide as an Electron Transport Layer",

abstract = "Planar perovskite solar cells using low-temperature atomic layer deposition (ALD) of the SnO2 electron transporting layer (ETL), with excellent electron extraction and hole-blocking ability, offer significant advantages compared with high-temperature deposition methods. The optical, chemical, and electrical properties of the ALD SnO2 layer and its influence on the device performance are investigated. It is found that surface passivation of SnO2 is essential to reduce charge recombination at the perovskite and ETL interface and show that the fabricated planar perovskite solar cells exhibit high reproducibility, stability, and power conversion efficiency of 20\%.",

keywords = "atomic layer deposition, passivation, perovskites, planar perovskite solar cells, SnO electron transporting layers",

author = "Yonghui Lee and Seunghwan Lee and Gabseok Seo and Sanghyun Paek and Cho, \{Kyung Taek\} and Huckaba, \{Aron J.\} and Marco Calizzi and Choi, \{Dong won\} and Park, \{Jin Seong\} and Dongwook Lee and Lee, \{Hyo Joong\} and Asiri, \{Abdullah M.\} and Nazeeruddin, \{Mohammad Khaja\}",

note = "Publisher Copyright: {\textcopyright} 2018 The Authors. Published by WILEY-VCH Verlag GmbH \& Co. KGaA, Weinheim",

year = "2018",

month = jun,

doi = "10.1002/advs.201800130",

language = "English",

volume = "5",

journal = "Advanced Science",

issn = "2198-3844",

number = "6",

}

TY - JOUR

T1 - Efficient Planar Perovskite Solar Cells Using Passivated Tin Oxide as an Electron Transport Layer

AU - Lee, Yonghui

AU - Lee, Seunghwan

AU - Seo, Gabseok

AU - Paek, Sanghyun

AU - Cho, Kyung Taek

AU - Huckaba, Aron J.

AU - Calizzi, Marco

AU - Choi, Dong won

AU - Park, Jin Seong

AU - Lee, Dongwook

AU - Lee, Hyo Joong

AU - Asiri, Abdullah M.

AU - Nazeeruddin, Mohammad Khaja

PY - 2018/6

Y1 - 2018/6

N2 - Planar perovskite solar cells using low-temperature atomic layer deposition (ALD) of the SnO2 electron transporting layer (ETL), with excellent electron extraction and hole-blocking ability, offer significant advantages compared with high-temperature deposition methods. The optical, chemical, and electrical properties of the ALD SnO2 layer and its influence on the device performance are investigated. It is found that surface passivation of SnO2 is essential to reduce charge recombination at the perovskite and ETL interface and show that the fabricated planar perovskite solar cells exhibit high reproducibility, stability, and power conversion efficiency of 20%.

AB - Planar perovskite solar cells using low-temperature atomic layer deposition (ALD) of the SnO2 electron transporting layer (ETL), with excellent electron extraction and hole-blocking ability, offer significant advantages compared with high-temperature deposition methods. The optical, chemical, and electrical properties of the ALD SnO2 layer and its influence on the device performance are investigated. It is found that surface passivation of SnO2 is essential to reduce charge recombination at the perovskite and ETL interface and show that the fabricated planar perovskite solar cells exhibit high reproducibility, stability, and power conversion efficiency of 20%.

KW - atomic layer deposition

KW - passivation

KW - perovskites

KW - planar perovskite solar cells

KW - SnO electron transporting layers

UR - https://www.scopus.com/pages/publications/85044402803

U2 - 10.1002/advs.201800130

DO - 10.1002/advs.201800130

M3 - Journal article

AN - SCOPUS:85044402803

SN - 2198-3844

VL - 5

JO - Advanced Science

JF - Advanced Science

IS - 6

M1 - 1800130

ER -

Efficient Planar Perovskite Solar Cells Using Passivated Tin Oxide as an Electron Transport Layer

Abstract

UN SDGs

Keywords

Quacquarelli Symonds(QS) Subject Topics

Access to Document

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