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Facile titanium(IV) chloride and TBD-mediated synthesis of N-aryl-substituted azacycles from arylhydrazines

  • Van Hieu Tran
  • , Wan Pyo Hong*
  • , Hee Kwon Kim*
  • *Corresponding author for this work
  • Jeonbuk National University
  • Gachon University

Research output: Contribution to journalJournal articlepeer-review

Abstract

A novel practical synthesis of N-aryl-substituted azacycles from arylhydrazines is described. In this method, target azacycles were prepared via reaction of arylhydrazines with cyclic ethers in the presence of both titanium(IV) chloride and 1,5,7-triazabicyclo[4.4.0]dec-5-ene (TBD) as key combined reagents. Using this synthetic protocol with titanium(IV) chloride and TBD, reaction of arylhydrazines with cyclic ethers successfully afforded various N-aryl-substituted azacycles in high yield. This facile synthetic method using arylhydrazines will be a promising guide for the synthesis of azacycles from arylhydrazines.

Original languageEnglish
Pages (from-to)777-783
Number of pages7
JournalBulletin of the Korean Chemical Society
Volume43
Issue number6
DOIs
StatePublished - 2022.06

Keywords

  • arylhydrazines
  • azacycles
  • heterocycles
  • Lewis acids
  • titanium(IV) chloride

Quacquarelli Symonds(QS) Subject Topics

  • Chemistry

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