Highly efficient and stable planar perovskite solar cells with reduced graphene oxide nanosheets as electrode interlayer

Jun Seok Yeo; Rira Kang; Sehyun Lee; Ye Jin Jeon; No Soung Myoung; Chang Lyoul Lee; Dong Yu Kim; Jin Mun Yun; You Hyun Seo; Seok Soon Kim; Seok In Na

doi:10.1016/j.nanoen.2014.12.022

Highly efficient and stable planar perovskite solar cells with reduced graphene oxide nanosheets as electrode interlayer

Jun Seok Yeo
, Rira Kang
, Sehyun Lee
, Ye Jin Jeon
, No Soung Myoung
, Chang Lyoul Lee
, Dong Yu Kim^*
, Jin Mun Yun
, You Hyun Seo
, Seok Soon Kim
, Seok In Na

^*Corresponding author for this work

Department of Flexible and Printable Electronics

Research output: Contribution to journal › Journal article › peer-review

351 Scopus citations

Abstract

We demonstrate a simple solution and room-temperature processed reduced graphene oxide (RGO) as a novel hole-transporting material (HTM) to guarantee highly efficient and highly stable CH₃NH₃PbI₃ perovskite solar cells (PeSCs). The effects of RGO HTM are systemically investigated in terms of PeSC efficiency, PeSC stability, morphology of perovskite film, recombination dynamics, and charge-transport through CH₃NH₃PbI₃/HTM interface. The resultant PeSC with a planar configuration of glass/ITO/RGO/CH₃NH₃PbI₃/PC₆₁BM/bathocuproine (BCP)/Ag exhibits improved device efficiency (maximum PCE of 10.8%) with high reproducibility than those of the reference devices using conventional PEDOT:PSS and GO HTMs. Also, the RGO-based PeSCs show highly desirable device stability in comparison to the PEDOT:PSS PeSCs.

Original language	English
Pages (from-to)	96-104
Number of pages	9
Journal	Nano Energy
Volume	12
DOIs	https://doi.org/10.1016/j.nanoen.2014.12.022
State	Published - 2015.03.1

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

SDG 7 Affordable and Clean Energy

Keywords

Interlayers
Perovskite solar cells
Planar structures
Reduced graphene oxides

Quacquarelli Symonds(QS) Subject Topics

Materials Science
Engineering - Electrical & Electronic
Engineering - Petroleum

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10.1016/j.nanoen.2014.12.022

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@article{4429aa8329ea48f9a6c9c00ce3b3e9b9,

title = "Highly efficient and stable planar perovskite solar cells with reduced graphene oxide nanosheets as electrode interlayer",

abstract = "We demonstrate a simple solution and room-temperature processed reduced graphene oxide (RGO) as a novel hole-transporting material (HTM) to guarantee highly efficient and highly stable CH3NH3PbI3 perovskite solar cells (PeSCs). The effects of RGO HTM are systemically investigated in terms of PeSC efficiency, PeSC stability, morphology of perovskite film, recombination dynamics, and charge-transport through CH3NH3PbI3/HTM interface. The resultant PeSC with a planar configuration of glass/ITO/RGO/CH3NH3PbI3/PC61BM/bathocuproine (BCP)/Ag exhibits improved device efficiency (maximum PCE of 10.8\%) with high reproducibility than those of the reference devices using conventional PEDOT:PSS and GO HTMs. Also, the RGO-based PeSCs show highly desirable device stability in comparison to the PEDOT:PSS PeSCs.",

keywords = "Interlayers, Perovskite solar cells, Planar structures, Reduced graphene oxides",

author = "Yeo, \{Jun Seok\} and Rira Kang and Sehyun Lee and Jeon, \{Ye Jin\} and Myoung, \{No Soung\} and Lee, \{Chang Lyoul\} and Kim, \{Dong Yu\} and Yun, \{Jin Mun\} and Seo, \{You Hyun\} and Kim, \{Seok Soon\} and Na, \{Seok In\}",

note = "Publisher Copyright: {\textcopyright} 2014 Elsevier Ltd.",

year = "2015",

month = mar,

day = "1",

doi = "10.1016/j.nanoen.2014.12.022",

language = "English",

volume = "12",

pages = "96--104",

journal = "Nano Energy",

issn = "2211-2855",

}

TY - JOUR

T1 - Highly efficient and stable planar perovskite solar cells with reduced graphene oxide nanosheets as electrode interlayer

AU - Yeo, Jun Seok

AU - Kang, Rira

AU - Lee, Sehyun

AU - Jeon, Ye Jin

AU - Myoung, No Soung

AU - Lee, Chang Lyoul

AU - Kim, Dong Yu

AU - Yun, Jin Mun

AU - Seo, You Hyun

AU - Kim, Seok Soon

AU - Na, Seok In

PY - 2015/3/1

Y1 - 2015/3/1

N2 - We demonstrate a simple solution and room-temperature processed reduced graphene oxide (RGO) as a novel hole-transporting material (HTM) to guarantee highly efficient and highly stable CH3NH3PbI3 perovskite solar cells (PeSCs). The effects of RGO HTM are systemically investigated in terms of PeSC efficiency, PeSC stability, morphology of perovskite film, recombination dynamics, and charge-transport through CH3NH3PbI3/HTM interface. The resultant PeSC with a planar configuration of glass/ITO/RGO/CH3NH3PbI3/PC61BM/bathocuproine (BCP)/Ag exhibits improved device efficiency (maximum PCE of 10.8%) with high reproducibility than those of the reference devices using conventional PEDOT:PSS and GO HTMs. Also, the RGO-based PeSCs show highly desirable device stability in comparison to the PEDOT:PSS PeSCs.

AB - We demonstrate a simple solution and room-temperature processed reduced graphene oxide (RGO) as a novel hole-transporting material (HTM) to guarantee highly efficient and highly stable CH3NH3PbI3 perovskite solar cells (PeSCs). The effects of RGO HTM are systemically investigated in terms of PeSC efficiency, PeSC stability, morphology of perovskite film, recombination dynamics, and charge-transport through CH3NH3PbI3/HTM interface. The resultant PeSC with a planar configuration of glass/ITO/RGO/CH3NH3PbI3/PC61BM/bathocuproine (BCP)/Ag exhibits improved device efficiency (maximum PCE of 10.8%) with high reproducibility than those of the reference devices using conventional PEDOT:PSS and GO HTMs. Also, the RGO-based PeSCs show highly desirable device stability in comparison to the PEDOT:PSS PeSCs.

KW - Interlayers

KW - Perovskite solar cells

KW - Planar structures

KW - Reduced graphene oxides

UR - https://www.scopus.com/pages/publications/84920742405

U2 - 10.1016/j.nanoen.2014.12.022

DO - 10.1016/j.nanoen.2014.12.022

M3 - Journal article

AN - SCOPUS:84920742405

SN - 2211-2855

VL - 12

SP - 96

EP - 104

JO - Nano Energy

JF - Nano Energy

ER -

Highly efficient and stable planar perovskite solar cells with reduced graphene oxide nanosheets as electrode interlayer

Abstract

UN SDGs

Keywords

Quacquarelli Symonds(QS) Subject Topics

Access to Document

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