Abstract
High-efficient red emission in III-nitride semiconductors remains a significant challenge due to crystal degradation caused by high In content and non-radiative recombination. In this study, we propose a 405 nm laser-induced re-crystallization (Re-Cryst) process to enhance the optical performance of 665 nm red-emitting core-shell InGaN/GaN nanowires grown by metal-organic chemical vapor deposition. Unlike conventional thermal annealing, this laser-based approach enables localized defect healing and improved lattice ordering while minimizing In decomposition. Micro-photoluminescence measurements revealed a 1.92-fold increase in band edge emission intensity at a shifted peak wavelength of 624 nm, attributed to strain relaxation and partial In decomposition. To evaluate the improvement in radiative recombination, we introduce a new figure of merit, referred to as the Radiative-PL-Rate (RRPL), which is defined as the rate of PL intensity at low excitation to that at saturation. The RRPL increased from 6.21% in the as-grown sample to 11.59% in the Re-Cryst sample, indicating a substantial suppression of non-radiative recombination. Furthermore, we demonstrated the mechanisms behind improved crystal quality and radiative efficiency, showing that the Re-Cryst process selectively heals defects, enhances red emission, and advances high-performance micro-displays for next-generation AR/VR applications.
| Original language | English |
|---|---|
| Article number | e03711 |
| Journal | Advanced Optical Materials |
| Volume | 14 |
| Issue number | 8 |
| DOIs | |
| State | Published - 2026.02.23 |
Keywords
- Core-shell nanowire
- InGaN
- Re-crystallization
- Red
- radiative-PL-Rate
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