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Localized Laser Recrystallization as an Alternative Route to High-Efficiency Red InGaN Nanowires

  • Sung Un Kim
  • , Yong Ho Kim
  • , Jeong Kyun Oh
  • , Sang Wook Lee
  • , Min Seok Lee
  • , Jae Hong Ju
  • , Se Bee Shin
  • , Jong Su Kim
  • , Bagavath Chandran
  • , Cheul Ro Lee*
  • , Dae Young Um*
  • , Yong Ho Ra*
  • *Corresponding author for this work

Research output: Contribution to journalJournal articlepeer-review

Abstract

High-efficient red emission in III-nitride semiconductors remains a significant challenge due to crystal degradation caused by high In content and non-radiative recombination. In this study, we propose a 405 nm laser-induced re-crystallization (Re-Cryst) process to enhance the optical performance of 665 nm red-emitting core-shell InGaN/GaN nanowires grown by metal-organic chemical vapor deposition. Unlike conventional thermal annealing, this laser-based approach enables localized defect healing and improved lattice ordering while minimizing In decomposition. Micro-photoluminescence measurements revealed a 1.92-fold increase in band edge emission intensity at a shifted peak wavelength of 624 nm, attributed to strain relaxation and partial In decomposition. To evaluate the improvement in radiative recombination, we introduce a new figure of merit, referred to as the Radiative-PL-Rate (RRPL), which is defined as the rate of PL intensity at low excitation to that at saturation. The RRPL increased from 6.21% in the as-grown sample to 11.59% in the Re-Cryst sample, indicating a substantial suppression of non-radiative recombination. Furthermore, we demonstrated the mechanisms behind improved crystal quality and radiative efficiency, showing that the Re-Cryst process selectively heals defects, enhances red emission, and advances high-performance micro-displays for next-generation AR/VR applications.

Original languageEnglish
Article numbere03711
JournalAdvanced Optical Materials
Volume14
Issue number8
DOIs
StatePublished - 2026.02.23

Keywords

  • Core-shell nanowire
  • InGaN
  • Re-crystallization
  • Red
  • radiative-PL-Rate

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