Mechanisms for Hydrolysis of Silicon Nanomembranes as Used in Bioresorbable Electronics

Lan Yin; Amir Barati Farimani; Kyoungmin Min; Nandigana Vishal; Jasper Lam; Yoon Kyeung Lee; Narayana R. Aluru; John A. Rogers

doi:10.1002/adma.201404579

Mechanisms for Hydrolysis of Silicon Nanomembranes as Used in Bioresorbable Electronics

Lan Yin
, Amir Barati Farimani
, Kyoungmin Min
, Nandigana Vishal
, Jasper Lam
, Yoon Kyeung Lee
, Narayana R. Aluru^*
, John A. Rogers

^*Corresponding author for this work

Electronic Materials Engineering

University of Illinois at Urbana-Champaign

Research output: Contribution to journal › Journal article › peer-review

111 Scopus citations

Abstract

Systematic experimental and theoretical studies of the hydrolysis of silicon nanomembranes at near-neutral pH conditions reveal the roles of anion concentration and temperature. An empirical model captures the dependence of the dissolution rates on key factors, and atomic-level simulations provide insights into the underlying chemistry.

Original language	English
Pages (from-to)	1857-1864
Number of pages	8
Journal	Advanced Materials
Volume	27
Issue number	11
DOIs	https://doi.org/10.1002/adma.201404579
State	Published - 2015.03.18

Keywords

density functional theory (DFT)
hydrolysis
molecular dynamics (MD)
silicon nanomembranes
transient electronics

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10.1002/adma.201404579

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title = "Mechanisms for Hydrolysis of Silicon Nanomembranes as Used in Bioresorbable Electronics",

abstract = "Systematic experimental and theoretical studies of the hydrolysis of silicon nanomembranes at near-neutral pH conditions reveal the roles of anion concentration and temperature. An empirical model captures the dependence of the dissolution rates on key factors, and atomic-level simulations provide insights into the underlying chemistry.",

keywords = "density functional theory (DFT), hydrolysis, molecular dynamics (MD), silicon nanomembranes, transient electronics",

author = "Lan Yin and Farimani, \{Amir Barati\} and Kyoungmin Min and Nandigana Vishal and Jasper Lam and Lee, \{Yoon Kyeung\} and Aluru, \{Narayana R.\} and Rogers, \{John A.\}",

note = "Publisher Copyright: {\textcopyright} 2015 Wiley-VCH Verlag GmbH \& Co. KGaA.",

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T1 - Mechanisms for Hydrolysis of Silicon Nanomembranes as Used in Bioresorbable Electronics

AU - Yin, Lan

AU - Farimani, Amir Barati

AU - Min, Kyoungmin

AU - Vishal, Nandigana

AU - Lam, Jasper

AU - Lee, Yoon Kyeung

AU - Aluru, Narayana R.

AU - Rogers, John A.

PY - 2015/3/18

Y1 - 2015/3/18

N2 - Systematic experimental and theoretical studies of the hydrolysis of silicon nanomembranes at near-neutral pH conditions reveal the roles of anion concentration and temperature. An empirical model captures the dependence of the dissolution rates on key factors, and atomic-level simulations provide insights into the underlying chemistry.

AB - Systematic experimental and theoretical studies of the hydrolysis of silicon nanomembranes at near-neutral pH conditions reveal the roles of anion concentration and temperature. An empirical model captures the dependence of the dissolution rates on key factors, and atomic-level simulations provide insights into the underlying chemistry.

KW - density functional theory (DFT)

KW - hydrolysis

KW - molecular dynamics (MD)

KW - silicon nanomembranes

KW - transient electronics

UR - https://www.scopus.com/pages/publications/84924855212

U2 - 10.1002/adma.201404579

DO - 10.1002/adma.201404579

M3 - Journal article

C2 - 25626856

AN - SCOPUS:84924855212

SN - 0935-9648

VL - 27

SP - 1857

EP - 1864

JO - Advanced Materials

JF - Advanced Materials

IS - 11

ER -

Mechanisms for Hydrolysis of Silicon Nanomembranes as Used in Bioresorbable Electronics

Abstract

Keywords

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